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Butane-to-Syngas Processing in Novel Micro-Reactors: Experimental Investigation of Butane Reforming for Solid Oxide Fuel Cell-based Small-Scale Powerplants - Softcover
This work investigates the production of syngas from butane by rhodium doped ceria/zirconia nanoparticles. The main issue of this study is to improve the catalytic performance at intermediate temperatures of 550°C. In the range of 500 to 600°C, a packed bed reactor with catalyst nanoparticles of 2.0 wt% Rh loading and silica-based plugs achieves nearly complete butane conversion with a hydrogen yield of 77%. In a next step, the production of syngas from butane is investigated by using a disk-shaped packed bed reactor containing Rh/ceria/zirconia nanoparticles at 550°C. Disk-shaped reactors achieve high hydrogen (92%) and carbon monoxide (82%) selectivities and complete butane conversion. This increased catalytic performance is due to a remarkably high contribution of Steam Reforming and Dry Reforming following Total Oxidation next to initial Partial Oxidation. Finally, a novel method is introduced to fabricate a ceramic foam containing catalytic nanoparticles by a direct and one-step sol-gelation procedure. The present dissertation proves that the catalyst is well suited to provide small portable butane processing units for applications in combination with micro fuel cells.
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Dr. sc. ETH Zurich, Dipl. Masch.-Ing. ETH: Diploma(2005) and Doctorate (2008) in Mechanical Engineering from ETHZurich, Switzerland. Since 2009 Postdoctoral Research Fellow atUniversity of California at Berkeley, USA.
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- PublisherSüdwestdeutscher Verlag für Hochschulschriften
- Publication date2009
- ISBN 10 3838107012
- ISBN 13 9783838107011
- BindingPaperback
- Number of pages100
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Butane-to-Syngas Processing in Novel Micro-Reactors: Experimental Investigation of Butane Reforming for Solid Oxide Fuel Cell-based Small-Scale Powerplants
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Butane-To-Syngas Processing in Novel Micro-Reactors
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Book Description Taschenbuch. Condition: Neu. This item is printed on demand - it takes 3-4 days longer - Neuware -This work investigates the production of syngas from butane by rhodium doped ceria/zirconia nanoparticles. The main issue of this study is to improve the catalytic performance at intermediate temperatures of 550°C. In the range of 500 to 600°C, a packed bed reactor with catalyst nanoparticles of 2.0 wt% Rh loading and silica-based plugs achieves nearly complete butane conversion with a hydrogen yield of 77%. In a next step, the production of syngas from butane is investigated by using a disk-shaped packed bed reactor containing Rh/ceria/zirconia nanoparticles at 550°C. Disk-shaped reactors achieve high hydrogen (92%) and carbon monoxide (82%) selectivities and complete butane conversion. This increased catalytic performance is due to a remarkably high contribution of Steam Reforming and Dry Reforming following Total Oxidation next to initial Partial Oxidation. Finally, a novel method is introduced to fabricate a ceramic foam containing catalytic nanoparticles by a direct and one-step sol-gelation procedure. The present dissertation proves that the catalyst is well suited to provide small portable butane processing units for applications in combination with micro fuel cells. 100 pp. Deutsch. Seller Inventory # 9783838107011
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ButanetoSyngas Processing in Novel MicroReactors Experimental Investigation of Butane Reforming for Solid Oxide Fuel Cellbased SmallScale Powerplants
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Butane-to-Syngas Processing in Novel Micro-Reactors : Experimental Investigation of Butane Reforming for Solid Oxide Fuel Cell-based Small-Scale Powerplants
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Book Description Taschenbuch. Condition: Neu. nach der Bestellung gedruckt Neuware - Printed after ordering - This work investigates the production of syngas from butane by rhodium doped ceria/zirconia nanoparticles. The main issue of this study is to improve the catalytic performance at intermediate temperatures of 550°C. In the range of 500 to 600°C, a packed bed reactor with catalyst nanoparticles of 2.0 wt% Rh loading and silica-based plugs achieves nearly complete butane conversion with a hydrogen yield of 77%. In a next step, the production of syngas from butane is investigated by using a disk-shaped packed bed reactor containing Rh/ceria/zirconia nanoparticles at 550°C. Disk-shaped reactors achieve high hydrogen (92%) and carbon monoxide (82%) selectivities and complete butane conversion. This increased catalytic performance is due to a remarkably high contribution of Steam Reforming and Dry Reforming following Total Oxidation next to initial Partial Oxidation. Finally, a novel method is introduced to fabricate a ceramic foam containing catalytic nanoparticles by a direct and one-step sol-gelation procedure. The present dissertation proves that the catalyst is well suited to provide small portable butane processing units for applications in combination with micro fuel cells. Seller Inventory # 9783838107011
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ButanetoSyngas Processing in Novel MicroReactors Experimental Investigation of Butane Reforming for Solid Oxide Fuel Cellbased SmallScale Powerplants
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(2009)
ISBN 10: 3838107012
ISBN 13: 9783838107011
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Butane-to-Syngas Processing in Novel Micro-Reactors
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