Long-Term Interactions of Full-Scale Cemented Waste Simulates with Salt Brines

Language: English

Published by Karlsruher Institut Für Technologie, 2017

3731505762 / 9783731505761

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Druck auf Anfrage Neuware - Printed after ordering - Since 1967 radioactive wastes have been disposed of in the Asse II salt mine in Northern Germany. A signifi-cant part of these wastes originated from the pilot reprocessing plant WAK in Karlsruhe and consisted of cemented NaNO3 solutions bearing fission products, actinides, as well as process chemicals. With respect to the long-term behavior of these wastes, the licensing authorities requested leaching experiments with full scale samples in relevant salt solutions which were performed since 1979. The experiments aimed at demonstrating the transferability of results obtained with laboratory samples to real waste forms and at the investigation of the effects of the industrial cementation process on the properties of the waste forms. This research program lasted until 2013. The corroding salt solutions were sampled several times and after termination of the experiments, the solid materials were analyzed by various methods. The results present-ed in this report cover the evolution of the solutions and the chemical and mineralogical characterization of the solids including radionuclides and waste components, and the paragenesis of solid phases (corrosion products). The outcome is compared to the results of model calculations. For safety analysis, conclusions are drawn on radionuclide retention, evolution of the geochemical environment, evolution of the density of solutions, and effects of temperature and porosity of the cement waste simulates on cesium mobilization.

Seller Inventory # 9783731505761

Title
Long-Term Interactions of Full-Scale Cemented Waste Simulates with Salt Brines
Author
Bernhard Kienzler
Publisher
Karlsruher Institut Für Technologie
Publication year
2017
Condition
Neu
Binding
Taschenbuch
Language
English
ISBN 10
3731505762
ISBN 13
9783731505761
Item weight
321 grams
Dimensions
297x210x7 mm

AHA-BUCH GmbH

Einbeck, Germany

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